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A logic-based controller for the mitigation of ventilation air methane in a catalytic flow reversal reactor

Zhikai LI, Zhangfeng QIN, Yagang ZHANG, Zhiwei WU, Hui WANG, Shuna LI, Mei DONG, Weibin FAN, Jianguo WANG

《化学科学与工程前沿（英文）》 2013年 第7卷 第3期   页码 347-356 doi: 10.1007/s11705-013-1347-0

摘要： The control system of a catalytic flow reversal reactor (CFRR) for the mitigation of ventilation air methane was investigated. A one-dimensional heterogeneous model with a logic-based controller was applied to simulate the CFRR. The simulation results indicated that the controller developed in this work performs well under normal conditions. Air dilution and auxiliary methane injection are effective to avoid the catalyst overheating and reaction extinction caused by prolonged rich and lean feed conditions, respectively. In contrast, the reactor is prone to lose control by adjusting the switching time solely. Air dilution exhibits the effects of two contradictory aspects on the operation of CFRR, i.e., cooling the bed and accumulating heat, though the former is in general more prominent. Lowering the reference temperature for flow reversal can decrease the bed temperature and benefit stable operation under rich methane feed condition.

关键词： ventilation air methane     reverse flow reactor     lean methane combustion     logic-based controller     mathematical modeling    

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Experimental study of humid air reverse diffusion combustion in a turbulent flow field

GE Bing, ZANG Shusheng, GU Xin

《能源前沿（英文）》 2007年 第1卷 第4期   页码 428-434 doi: 10.1007/s11708-007-0062-6

摘要： Experiments were performed to investigate the differences between the propane/air turbulent diffusion reactive flows past bluff-body and the propane/humid air turbulent diffusion reactive flows in the same conditions. The velocity

关键词： propane/humid     propane/air turbulent     bluff-body     turbulent diffusion    

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Nitrogen removal performance of municipal reverse osmosis concentrate with low C/N ratio by membrane-aeratedbiofilm reactor

Xiao Quan, Kai Huang, Mei Li, Meichao Lan, Baoan Li

《环境科学与工程前沿（英文）》 2018年 第12卷 第6期 doi: 10.1007/s11783-018-1047-6

摘要：

MABR exhibits excellent TN removal performance for treating ROC with low C/N ratio.

Operating conditions should be properly controlled to achieve optimal TN removal.

Denitrifying bacteria and NOB are proved notably inhibited by high salinity stress.

The TN removal rate remains over 70% when the NaCl addition amount is below 20 g/L.

关键词： Membrane-aerated biofilm reactor (MABR)     Salinity     Total nitrogen     Reverse osmosis concentrate    

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Experimental study of critical flow of water at supercritical pressure

Yuzhou CHEN, Chunsheng YANG, Shuming ZHANG, Minfu ZHAO, Kaiwen DU, Xu CHENG

《能源前沿（英文）》 2009年 第3卷 第2期   页码 175-180 doi: 10.1007/s11708-009-0029-6

摘要： Experimental studies of the critical flow of water were conducted under steady-state conditions with a nozzle 1.41 mm in diameter and 4.35 mm in length, covering the inlet pressure range of 22.1-26.8 MPa and inlet temperature range of 38-474°C. The parametric trend of the flow rate was investigated, and the experimental data were compared with the predictions of the homogeneous equilibrium model, the Bernoulli correlation, and the models used in the reactor safety analysis code RELAP5/MOD3.3. It is concluded that in the near or beyond pseudo-critical region, thermal-dynamic equilibrium is dominant, and at a lower temperature, choking does not occur. The onset of the choking condition is not predicted reasonably by the RELAP5 code.

关键词： critical flow     supercritical water-cooled reactor(SCWR)     reactor safety     loss of coolant accident(LOCA)    

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Theoretical study on flow and radiation in tubular solar photocatalytic reactor

《能源前沿（英文）》 2021年 第15卷 第3期   页码 687-699 doi: 10.1007/s11708-021-0773-9

摘要： In this paper, based on the mixture flow model, an optimized six-flux model is first established and applied to the tubular solar photocatalytic reactor. Parameters influencing photocatalyst distribution and radiation distribution at the reactor outlet, viz. catalyst concentration and circulation speed, are also analyzed. It is found that, at the outlet of the reactor, the optimized six-flux model has better performances (the energy increase by 1900% and 284%, respectively) with a higher catalyst concentration (triple) and a lower speed (one third).

关键词： photocatalytic hydrogen photoreactor     nume- rical simulation     solar energy     flow model     radiation model    

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CFD simulation of the hydrodynamics in an internal air-lift reactor with two different configurations

Mona EBRAHIMIFAKHAR, Elmira MOHSENZADEH, Sadegh MORADI, Mostafa MORAVEJI, Mahmoud SALIMI

《化学科学与工程前沿（英文）》 2011年 第5卷 第4期   页码 455-462 doi: 10.1007/s11705-011-1116-x

摘要： Computational fluid dynamics (CFD) was used to investigate the hydrodynamic parameters of two internal airlift bioreactors with different configurations. Both had a riser diameter of 0.1 m. The model was used to predict the effect of the reactor geometry on the reactor hydrodynamics. Water was utilized as the continuous phase and air in the form of bubbles was applied as the dispersed phase. A two-phase flow model provided by the bubbly flow application mode was employed in this project. In the liquid phase, the turbulence can be described using the - model. Simulated gas holdup and liquid circulation velocity results were compared with experimental data. The predictions of the simulation are in good agreement with the experimental data.

关键词： airlift reactor     gas holdup     liquid circulation velocity     bubbly flow     computational fluid dynamics (CFD)    

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Enhanced methane recovery and exoelectrogen-methanogen evolution from low-strength wastewater in an up-flowbiofilm reactor with conductive granular graphite fillers

Zechong Guo, Lei Gao, Ling Wang, Wenzong Liu, Aijie Wang

《环境科学与工程前沿（英文）》 2018年 第12卷 第4期 doi: 10.1007/s11783-018-1074-3

摘要：

Methane yield increased 22 times from low-strength wastewater by applying conductive fillers.

Conductive fillers accelerated the start-up stage of anaerobic biofilm reactor.

Conductive fillers altered methanogens structure.

关键词： Low-strength wastewater     Methane production     Conductive filler     Microbial community structure    

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Highly hydrophobic oil−water separation membrane: reutilization of waste reverse osmosis membrane

《化学科学与工程前沿（英文）》 2023年 第17卷 第10期   页码 1606-1615 doi: 10.1007/s11705-022-2200-0

摘要： The increasing applications of seawater desalination technology have led to the wide usage of polyamide reverse osmosis membranes, resulting in a large number of wasted reverse osmosis membranes. In this work, the base nonwoven layer of the wasted reverse osmosis membrane was successfully modified into the hydrophobic membrane via surface deposition strategy including TiO2 and 1H,1H,2H,2H-perfluorooctyltrichlorosilane (PFOTS), respectively. Various techniques were applied to characterize the obtained membranes, which were then used to separate the oil–water system. The optimally modified membrane displayed good hydrophobicity with a contact angle of 135.2° ± 0.3°, and its oil–water separation performance was as high as 97.8%. After 20 recycle tests, the oil–water separation performance remained more than 96%, which was attributed to the film adhesion of the anchored TiO2 and PFOTS layer on the surface. This work might provide a new avenue for recycling the wasted reverse osmosis membrane used in oily wastewater purification.

关键词： oil–water separation     wasted reverse osmosis membrane     hydrophobic modification    

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Centrifuge experiments for shallow tunnels at active reverse fault intersection

Mehdi SABAGH, Abbas GHALANDARZADEH

《结构与土木工程前沿（英文）》 2020年 第14卷 第3期   页码 731-745 doi: 10.1007/s11709-020-0614-7

摘要： Tunnels extend in large stretches with continuous lengths of up to hundreds of kilometers which are vulnerable to faulting in earthquake-prone areas. Assessing the interaction of soil and tunnel at an intersection with an active fault during an earthquake can be a beneficial guideline for tunnel design engineers. Here, a series of 4 centrifuge tests are planned and tested on continuous tunnels. Dip-slip surface faulting in reverse mechanism of 60-degree is modeled by a fault simulator box in a quasi-static manner. Failure mechanism, progression and locations of damages to the tunnels are assessed through a gradual increase in Permanent Ground Displacement (PGD). The ground surface deformations and strains, fault surface trace, fault scarp and the sinkhole caused by fault movement are observed here. These ground surface deformations are major threats to stability, safety and serviceability of the structures. According to the observations, the modeled tunnels are vulnerable to reverse fault rupture and but the functionality loss is not abrupt, and the tunnel will be able to tolerate some fault displacements. By monitoring the progress of damage states by increasing PGD, the fragility curves corresponding to each damage state were plotted and interpreted in related figures.

关键词： reverse fault rupture     continuous tunnel     geotechnical centrifuge     ground surface deformations     fragility curves    

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Self-healing polyamide reverse osmosis membranes with temperature-responsive intelligent nanocontainers

《化学科学与工程前沿（英文）》 2023年 第17卷 第9期   页码 1183-1195 doi: 10.1007/s11705-022-2287-3

摘要： Improving the performance of reverse osmosis membranes remains great challenge to ensure excellent NaCl rejection while maintaining high water permeability and chlorine resistance. Herein, temperature-responsive intelligent nanocontainers are designed and constructed to improve water permeability and chlorine resistance of polyamide membranes. The nanocontainer is synthesized by layer-by-layer self-assembly with silver nanoparticles as the core, sodium alginate and chitosan as the repair materials, and polyvinyl alcohol as the shell. When the polyamide layer is damaged by chlorine attack, the polyvinyl alcohol shell layer dissolves under temperature stimulation of 37 °C, releasing inner sodium alginate and chitosan to repair broken amide bonds. The polyvinyl alcohol shell responds to temperature in line with actual operating environment, which can effectively synchronize the chlorination of membranes with temperature response and release inner materials to achieve self-healing properties. With adding temperature-responsive intelligent nanocontainers, the NaCl rejection of thin film composite membrane decreased by 15.64%, while that of thin film nanocomposite membrane decreased by only 8.35% after 9 chlorination cycles. Effective repair treatment and outstanding chlorine resistance as well as satisfactory stability suggest that temperature-responsive intelligent nanocontainer has great potential as membrane-doping material for the targeted repair of polyamide reverse osmosis membranes.

关键词： reverse osmosis     nanocontainer     self-healing     chlorine resistance     water permeability    

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Mechanism of ethanol/water reverse separation through a functional graphene membrane: a molecular simulation

《化学科学与工程前沿（英文）》 2023年 第17卷 第3期   页码 347-357 doi: 10.1007/s11705-022-2246-z

摘要： Reverse-selective membranes have attracted considerable interest for bioethanol production. However, to date, the reverse-separation performance of ethanol/water is poor and the separation mechanism is unclear. Graphene-based membranes with tunable apertures and functional groups have shown substantial potential for use in molecular separation. Using molecular dynamics simulations, for the first time, we reveal two-way selectivity in ethanol/water separation through functional graphene membranes. Pristine graphene (PG) exhibits reverse-selective behavior with higher ethanol fluxes than water, resulting from the preferential adsorption for ethanol. Color flow mappings show that this ethanol-permselective process is initiated by the presence of ethanol-enriched and water-barren pores; this has not been reported in previous studies. In contrast, water molecules are preferred for hydroxylated graphene membranes because of the synergistic effects of molecular sieving and functional-group attraction. A simulation of the operando condition shows that the PG membrane with an aperture size of 3.8 Å achieves good separation performance, with an ethanol/water separation factor of 34 and a flux value of 69.3 kg∙m‒2∙h‒1∙bar‒1. This study provides new insights into the reverse-selective mechanism of porous graphene membranes and a new avenue for efficient biofuel production.

关键词： reverse separation     graphene membrane     ethanol/water separation     molecular simulation    

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Tracing the impact of stack configuration on interface resistances in reverse electrodialysis by in situ

《环境科学与工程前沿（英文）》 2022年 第16卷 第4期 doi: 10.1007/s11783-021-1480-9

摘要：

• RED performance and stack resistance were studied by EIS and LSV.

关键词： Reverse electrodialysis     Electrochemical impedance spectroscopy     Concentration polarization     Spacer shadow effect    

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Preparation of reverse osmosis membrane with high permselectivity and anti-biofouling properties for

《环境科学与工程前沿（英文）》 2022年 第16卷 第7期 doi: 10.1007/s11783-021-1497-0

摘要：

• Nanoparticle incorporation and anti-biofouling grafting were integrated.

关键词： Anti-biofouling grafting     Nanoparticle incorporation     Sterilization rates     Water flux     Water flux recovery    

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Efficient production of hydrogen peroxide in microbial reverse-electrodialysis cells coupled with thermolytic

《环境科学与工程前沿（英文）》 2023年 第17卷 第9期 doi: 10.1007/s11783-023-1708-y

摘要：

● Appreciable H2O2 production rate was achieved in MRCs utilizing NH4HCO3 solutions.

关键词： Microbial reverse-electrodialysis cell     Hydrogen peroxide production     Ammonium bicarbonate     Electrolysis cell     Optimization    

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Surface-tailoring chlorine resistant materials and strategies for polyamide thin film composite reverse

《化学科学与工程前沿（英文）》 2022年 第16卷 第5期   页码 564-591 doi: 10.1007/s11705-021-2109-z

摘要： Polyamide thin film composite membranes have dominated current reverse osmosis market on account of their excellent separation performances compared to the integrally skinned counterparts. Despite their very promising separation performance, chlorine-induced degradation resulted from the susceptibility of polyamide toward chlorine attack has been regarded as the Achilles’s heel of polyamide thin film composite. The free chlorine species present during chlorine treatment can impair membrane performance through chlorination and depolymerization of the polyamide selective layer. From material point of view, a chemically stable membrane is crucial for the sustainable application of membrane separation process as it warrants a longer membrane lifespan and reduces the cost involved in membrane replacement. Various strategies, particularly those involved membrane material optimization and surface modifications, have been established to address this issue. This review discusses membrane degradation by free chlorine attack and its correlation with the surface chemistry of polyamide. The advancement in the development of chlorine resistant polyamide thin film composite membranes is reviewed based on the state-of-the-art surface modifications and tailoring approaches which include the in situ and post-fabrication membrane modifications using a broad range of functional materials. The challenges and future directions in this field are also highlighted.

关键词： reverse osmosis     polyamide     thin film composite membranes     chlorine resistance     surface modification    

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标题 作者 时间 类型 操作

A logic-based controller for the mitigation of ventilation air methane in a catalytic flow reversal reactor

Zhikai LI, Zhangfeng QIN, Yagang ZHANG, Zhiwei WU, Hui WANG, Shuna LI, Mei DONG, Weibin FAN, Jianguo WANG

期刊论文

Experimental study of humid air reverse diffusion combustion in a turbulent flow field

GE Bing, ZANG Shusheng, GU Xin

期刊论文

Nitrogen removal performance of municipal reverse osmosis concentrate with low C/N ratio by membrane-aeratedbiofilm reactor

Xiao Quan, Kai Huang, Mei Li, Meichao Lan, Baoan Li

期刊论文

Experimental study of critical flow of water at supercritical pressure

Yuzhou CHEN, Chunsheng YANG, Shuming ZHANG, Minfu ZHAO, Kaiwen DU, Xu CHENG

期刊论文

Theoretical study on flow and radiation in tubular solar photocatalytic reactor

期刊论文

CFD simulation of the hydrodynamics in an internal air-lift reactor with two different configurations

Mona EBRAHIMIFAKHAR, Elmira MOHSENZADEH, Sadegh MORADI, Mostafa MORAVEJI, Mahmoud SALIMI

期刊论文

Enhanced methane recovery and exoelectrogen-methanogen evolution from low-strength wastewater in an up-flowbiofilm reactor with conductive granular graphite fillers

Zechong Guo, Lei Gao, Ling Wang, Wenzong Liu, Aijie Wang

期刊论文

Highly hydrophobic oil−water separation membrane: reutilization of waste reverse osmosis membrane

期刊论文

Centrifuge experiments for shallow tunnels at active reverse fault intersection

Mehdi SABAGH, Abbas GHALANDARZADEH

期刊论文

Self-healing polyamide reverse osmosis membranes with temperature-responsive intelligent nanocontainers

期刊论文

Mechanism of ethanol/water reverse separation through a functional graphene membrane: a molecular simulation

期刊论文

Tracing the impact of stack configuration on interface resistances in reverse electrodialysis by in situ

期刊论文

Preparation of reverse osmosis membrane with high permselectivity and anti-biofouling properties for

期刊论文

Efficient production of hydrogen peroxide in microbial reverse-electrodialysis cells coupled with thermolytic

期刊论文

Surface-tailoring chlorine resistant materials and strategies for polyamide thin film composite reverse

期刊论文